I'm not sure if it's possible to truly liberate major factions, but looting their former capitol city and leaving it unguarded should cause the rebels to retake it and reform their nation. Only problem is you'll be at war with them which seems to be contrary to your goals. You could also try taking a few territories and then gifting them for peace/alliance/trade etc which could work, but that means defending all those territories in the meantime.
Good luck and nice work! +rep





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